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Process Modeling of Mineral Dissolution From Nano‐Scale Surface Topography Observations

GRL - Fri, 08/16/2024 - 07:39
Abstract

We present an innovative approach that combines a unique real-time data set documenting absolute dissolution rates of a calcite crystal with an original reactive transport model tailored to the analysis of the dynamics of nano-scale mineral dissolution processes. Providing robust and physically based fundamental understanding on the kinetics of mineral dissolution is at the core of various geo-engineered strategies to quantify chemical weathering patterns across diverse spatial and temporal scales. Here, we rely on data obtained through Atomic Force Microscopy. We provide a mathematical framework to describe three-dimensional dynamics of the mineral surface topography, and show convergence of the numerical approach for vertical grid spacing down to sub-nm resolution.

Historical Trends in Cold‐Season Mid‐Latitude Cyclones in the Great Lakes Region

GRL - Fri, 08/16/2024 - 06:44
Abstract

The Great Lakes Region (GLR) of North America is at the intersection of multiple extratropical cyclone (ETC) tracks, and the region's cold-season climate is heavily influenced by the large temperature gradients and intense precipitation associated with these cyclones. The goal of this study is to understand how ETCs are changing within a warming climate. Historical GLR cyclone characteristics from 1959 to 2021 are examined using a storm tracking algorithm and the ERA-5 atmospheric reanalysis. Of the 886 cyclones identified, half are the large long-track cyclones that are typically included in ETC studies, and half are smaller short-track cyclones that, while not always considered in ETC studies, still have an important impact on the GLR with significant precipitation trends. While all cyclones exhibit strong interannual variability, storm trajectories appear to be migrating northward and, most notably, the cyclones are becoming warmer and wetter at a rate faster than the background climate.

Exploring Uncertainty of Trends in the North Pacific Jet Position

GRL - Fri, 08/16/2024 - 06:24
Abstract

It has been difficult to establish trends in the observed jet streams, despite modeling studies suggesting they will move polewards in a warming world. While this is partly due to biases between the models and observations, we propose that another uncertainty is rooted in the choice of statistic used to determine the ‘jet latitude’ — one measure used to quantify the jet position. We use seven different jet latitude statistics, four climate reanalysis products, and CMIP6 simulations to assess the relative importance of different uncertainties associated with lower-tropospheric North Pacific Jet (NPJ) trends. Our results show a statistically significant poleward trend in the observed winter NPJ across all reanalyzes and using all jet latitude statistics. The magnitude of this trend is most sensitive to the choice of statistic. Furthermore, we find that the NPJ shifts poleward in Autumn under high emission scenarios, which is robust to the choice of jet statistic.

Reductions in Forest Resilience: Unraveling the Decoupling Between Gross Primary Productivity and Photosynthetic Efficiency

GRL - Fri, 08/16/2024 - 05:44
Abstract

Ecosystem-scale photosynthetic efficiency (EPE) is proposed as an effective indicator to quantify gross primary productivity (GPP), but how the coupling between EPE and GPP varies as vegetation resilience decreases has not been evaluated. Here, we quantified forest resilience with optimized Bayesian models. With the use of multisource satellite and modeling data, our study revealed that forests on the Loess Plateau and in the Qinba Mountains in China are experiencing rapid resilience loss and are already facing mortality warnings after 2010. Reductions in resilience also drove the marked decoupling of GPP from EPE. Notably, the decline in resilience was accompanied by a decrease in EPE in about 74% of the forests while GPP increased. The mechanism underlying this decoupling could be attributed to enhanced atmospheric water demand and soil water constraints. The dynamic relationships found here could help to improve forest mortality models and enhance photosynthesis-based GPP evaluation.

Multi‐Decadal Variability of Amundsen Sea Low Controlled by Natural Tropical and Anthropogenic Drivers

GRL - Fri, 08/16/2024 - 05:40
Abstract

A crucial factor influencing the mass balance of the West Antarctic Ice Sheet is the Amundsen Sea Low (ASL), a climatological low-pressure region situated off the West Antarctic coast. However, albeit the deepening of the ASL since the 1950s has been attributed to anthropogenic forcing, the multi-decadal variability of the ASL remains poorly understood, because of a lack of long observations. Here, we apply a newly developed data assimilation method to reconstruct the ASL over 1870–2000. We study the forced and internal variability of the ASL using our new reconstruction in concert with existing large ensembles of climate model simulations. Our findings robustly demonstrate that an atmospheric teleconnection originating from the tropical Indo-Pacific is the main driver of ASL variability at the multi-decadal time scale, with resemblance to the Interdecadal Pacific Oscillation. Since the mid-20th century, anthropogenic forcing has emerged as a dominant contributor to the strengthening of the ASL.

On the Tropical Cyclone Integrated Kinetic Energy Balance

GRL - Fri, 08/16/2024 - 05:40
Abstract

Current global historical reanalyzes prevent to adequately examine the role of the near-core surface wind structural properties on tropical cyclones climate trends. Here we provide theoretical and observational evidences that they are crucial for the monitoring of integrated kinetic energy. The kinetic energy balance is reduced to a simple rule involving two parameters characterizing the surface wind structure and directly suggested by the governing equations. The theory is uniquely verified with a database of high-resolution ocean surface winds estimated from all-weather spaceborne synthetic aperture radar. Such measurements provide indirect estimates of a multiplicative constant modulating the kinetic energy balance and associated with the system thermodynamics. Consequently, accumulated high-resolution acquisitions of the ocean surface shall allow to better monitor the integrated kinetic energy and provide new means to tackle climatological studies of tropical cyclones destructiveness.

Interactions and Multifrequency Radiation Characteristics of Bidirectional Leaders in Altitude‐Triggered Lightning

GRL - Fri, 08/16/2024 - 05:30
Abstract

Altitude-triggered lightning provides favorable conditions for the research of bidirectional leader system. In the summer of 2023, altitude-triggered lightning experiment was conducted on the Field Experiment Base on Lightning Sciences, China Meteorological Administration. The multifrequency radiation characteristics of bidirectional leaders and the interactions of both ends during the propagation are analyzed. Specifically, the discharge processes that produce LF-MF magnetic radiations from bidirectional leaders are revealed by high-speed images, and these LF-MF radiations correspond to the VHF radiations generated by bidirectional leaders well. Unlike the strong correlation between LF-MF radiation strengths and discharge intensities, the VHF radiation strengths exhibit significant variation even among similar-intensity discharge events, as VHF radiations correspond to the random and microscopic discharge processes associated with streamers. Furthermore, the changes in leader speed and channel brightness before and after the initiation of bidirectional leaders indicate that the development of the two ends of bidirectional leaders is mutually reinforcing.

Global Cloud Biases in Optical Satellite Remote Sensing of Rivers

GRL - Fri, 08/16/2024 - 05:20
Abstract

Satellite imagery provides a global perspective for studying river hydrology and water quality, but clouds remain a fundamental limitation of optical sensors. Explicit studies of this problem were limited to specific locations or regions. In this study, we characterize the global severity of this limitation by analyzing 22 years of daily satellite cloud cover data and modeled river discharge for a global sample 21,642 river reaches of diverse sizes and climates. Our results show that the bias in observed river discharge is highly organized in space, particularly affecting Tropical and Arctic rivers. Given the fundamental nature of this cloud limitation, optical satellites will always provide a biased representation of river conditions. We discuss several strategies to mitigate bias, including modeling, data fusion, and temporal averaging, yet these methods introduce their own challenges and uncertainties.

On the Physical Mechanisms Driving the Different Deep Penetration of Radiation Belt Electrons and Protons

JGR:Space physics - Fri, 08/16/2024 - 05:10
Abstract

During active geomagnetic periods both electrons and protons in the outer radiation belt have been frequently observed to penetrate to low L (<4). Previous studies have demonstrated systematic differences in the deep penetration of the two species of particles, most notably that the penetration of protons is observed less frequently than for electrons of the same energies. A recent study by Mei et al. (2023, https://doi.org/10.1029/2022GL101921) showed that the time-varying convection electric field contributes to the deeper penetration of low-energy electrons and that a radial diffusion-convection model can be used to reproduce the storm-time penetration of lower-energy electrons to lower L. In this study, we analyze and provide physical explanations for the different behaviors of electrons and protons in terms of their penetration depth to low L. A radial diffusion-convection model is applied for the two species with coefficients that are adjusted according to the mass-dependent relativistic effects on electron and proton drift velocity, and the different loss mechanisms included for each species. Electromagnetic ion cyclotron (EMIC) wave scattering losses for 100s of keV protons during a specific event are modeled and quantified; the results suggest that EMIC waves interacting with protons of lower energies than electrons can contribute to prevent the inward transport of the protons.

Mixing, Water Transformation, and Melting Close to a Tidewater Glacier

GRL - Fri, 08/16/2024 - 05:06
Abstract

Marine-terminating glacier fjords play a central role in the transport of oceanic heat toward ice sheets, regulating their melt. Mixing processes near glacial termini are key to this circulation but remain poorly understood. We present new summer measurements of circulation and mixing near a marine-terminating glacier with active sub-glacial discharge. 65% of the fjord's vertical overturning circulation is driven by the buoyant plume, however we newly report intense vertical and horizontal mixing in the plume's horizontal spreading phase, accounting for the remaining 35%. Buoyant plume theory supports 2%–5% of total glacial melt. Thus, most of the heat associated with vertical overturing short-circuits the glacial front. We find however that turbulence in the horizontal spreading phase redistributes the short-circuited heat back into the surface waters of the near-glacial zone. Our findings highlight the need for further research on the complex mixing processes that occur near the glacier terminus.

Observational Evidence for Three Time‐Scale Modulations in the Pulsating Aurora

GRL - Fri, 08/16/2024 - 04:39
Abstract

We report an Arase-all sky imager (ASI) conjugate event in which the pulsating aurora (PsA) has a one-to-one correspondence with chorus bursts. Wavelet analysis displayed three peaks at ∼0.3 Hz, 4 Hz, and >10 Hz, corresponding to the main pulsation, internal modulation, and fast modulation, respectively. These correspond to the old terms of ∼5–15 s pulsations, chorus risers/elements and subelements/subpackets, respectively. Electron “microbursts” correspond to the 4-Hz peak. The internal and fast modulations are further verified by the analysis based on fast Fourier transform analyses. Moreover, the spatial distributions of the Fourier spectral amplitude show that the internal and fast modulations are well-structured within auroral patches. The above results indicate a paradigm shift away from quasilinear theory which implicitly assumes diffuse wave generation. The three time-scale modulations are consistent with coherent chorus which has been theoretically argued to lead to pitch angle transport three orders of magnitude faster.

Implementation of a brittle sea ice rheology in an Eulerian, finite-difference, C-grid modeling framework: impact on the simulated deformation of sea ice in the Arctic

Geoscientific Model Development - Thu, 08/15/2024 - 18:47
Implementation of a brittle sea ice rheology in an Eulerian, finite-difference, C-grid modeling framework: impact on the simulated deformation of sea ice in the Arctic
Laurent Brodeau, Pierre Rampal, Einar Ólason, and Véronique Dansereau
Geosci. Model Dev., 17, 6051–6082, https://doi.org/10.5194/gmd-17-6051-2024, 2024
A new brittle sea ice rheology, BBM, has been implemented into the sea ice component of NEMO. We describe how a new spatial discretization framework was introduced to achieve this. A set of idealized and realistic ocean and sea ice simulations of the Arctic have been performed using BBM and the standard viscous–plastic rheology of NEMO. When compared to satellite data, our simulations show that our implementation of BBM leads to a fairly good representation of sea ice deformations.

A simple approach to represent precipitation-derived freshwater fluxes into nearshore ocean models: an FVCOM4.1 case study of Quatsino Sound, British Columbia

Geoscientific Model Development - Thu, 08/15/2024 - 18:47
A simple approach to represent precipitation-derived freshwater fluxes into nearshore ocean models: an FVCOM4.1 case study of Quatsino Sound, British Columbia
Krysten Rutherford, Laura Bianucci, and William Floyd
Geosci. Model Dev., 17, 6083–6104, https://doi.org/10.5194/gmd-17-6083-2024, 2024
Nearshore ocean models often lack complete information about freshwater fluxes due to numerous ungauged rivers and streams. We tested a simple rain-based hydrological model as inputs into an ocean model of Quatsino Sound, Canada, with the aim of improving the representation of the land–ocean connection in the nearshore model. Through multiple tests, we found that the performance of the ocean model improved when providing 60 % or more of the freshwater inputs from the simple runoff model.

TAMS: a tracking, classifying, and variable-assigning algorithm for mesoscale convective systems in simulated and satellite-derived datasets

Geoscientific Model Development - Thu, 08/15/2024 - 18:47
TAMS: a tracking, classifying, and variable-assigning algorithm for mesoscale convective systems in simulated and satellite-derived datasets
Kelly M. Núñez Ocasio and Zachary L. Moon
Geosci. Model Dev., 17, 6035–6049, https://doi.org/10.5194/gmd-17-6035-2024, 2024
TAMS is an open-source Python-based package for tracking and classifying mesoscale convective systems that can be used to study observed and simulated systems. Each step of the algorithm is described in this paper with examples showing how to make use of visualization and post-processing tools within the package. A unique and valuable feature of this tracker is its support for unstructured grids in the identification stage and grid-independent tracking.

Global sensitivity analysis of simulated remote sensing polarimetric observations over snow

Atmos. Meas. techniques - Thu, 08/15/2024 - 16:33
Global sensitivity analysis of simulated remote sensing polarimetric observations over snow
Matteo Ottaviani, Gabriel Harris Myers, and Nan Chen
Atmos. Meas. Tech., 17, 4737–4756, https://doi.org/10.5194/amt-17-4737-2024, 2024
We analyze simulated polarization observations over snow to investigate the capabilities of remote sensing to determine surface and atmospheric properties in snow-covered regions. Polarization measurements are demonstrated to aid in the determination of snow grain shape, ice crystal roughness, and the vertical distribution of impurities in the snow–atmosphere system, data that are critical for estimating snow albedo for use in climate models.

Drone CO2 measurements during the Tajogaite volcanic eruption

Atmos. Meas. techniques - Thu, 08/15/2024 - 16:33
Drone CO2 measurements during the Tajogaite volcanic eruption
John Ericksen, Tobias P. Fischer, G. Matthew Fricke, Scott Nowicki, Nemesio M. Pérez, Pedro Hernández Pérez, Eleazar Padrón González, and Melanie E. Moses
Atmos. Meas. Tech., 17, 4725–4736, https://doi.org/10.5194/amt-17-4725-2024, 2024
Volcanic eruptions emit significant quantities of carbon dioxide (CO2) to the atmosphere. We present a new method for directly determining the CO2 emission from a volcanic eruption on the island of La Palma, Spain, using an unpiloted aerial vehicle (UAV). We also collected samples of the emitted CO2 and analyzed their isotopic composition. Together with the emission rate the isotopic data provide valuable information on the state of volcanic activity and the potential evolution of the eruption.

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