Feed aggregator

Abstract

The occurrence of natural hydrogen and its sources have been reviewed extensively in the literature over the last few years, with current research across both academia and industry focused on assessing the feasibility of utilizing natural hydrogen as an energy resource. However, gaps remain in our understanding of the mechanisms responsible for the large-scale transport of hydrogen and migration through the deep and shallow Earth and within geological basins. Due to the unique chemical and physical properties of hydrogen, the timescales of migration within different areas of Earth vary from billions to thousands of years. Within the shallow Earth, diffusive and advective transport mechanisms are dependent on a wide range of parameters including geological structure, microbial activity, and subsurface environmental factors. Hydrogen migration through different media may occur from geological timescales to days and hours. We review the nature and timescale of hydrogen migration from the planetary to basin-scale, and within both the deep and shallow Earth. We explore the role of planetary accretion in setting the hydrogen budget of the lower mantle, discuss conceptual frameworks for primordial or deep mantle hydrogen migration to the Earth's surface and evaluate the literature on the lower mantle's potential role in setting the hydrogen budget of rocks delivered from the deep Earth. We also review the mechanisms and timescales of hydrogen within diffusive and advective, fossil versus generative and within biologically moderated systems within the shallow Earth. Finally, we summarize timescales of hydrogen migration through different regions within sedimentary basins.

Abstract

The identification of the Grenvillian-age ophiolite suites in the Yangtze block in recent years suggested that the northern Yangtze subblock (NYB) and the southern Yangtze subblock (SYB) were once separated by an ocean in late Mesoproterozoic. Although some paleogeographic models advocated the Pre-Grenvillian connections between the south China blocks and Laurentia, none of them has been paleomagnetically tested. Here we report the new paleomagnetic results obtained from the ∼1,270 Ma purplish-red muddy dolomite beds of the Luanshigou Formation, Shennongjia Group, NYB, providing new constraints for reconstructing the paleogeographic positions of the south China blocks in late Mesoproterozoic. A total of 447 samples underwent stepwise thermal demagnetization. Two components were identified. The low-temperature component is interpreted as the recent viscous remnant magnetization. The high-temperature component was obtained from 64 samples below 580°C and from 177 samples below 690°C, directed northeast-up or southwest-down, antipodally, positioning the paleomagnetic pole at 18.5°S, 74.4°E (dm/dp = 2.5/1.6°). Rock magnetic results demonstrate that the magnetic carriers in purplish-red dolomite and pale-pink dolomite are predominated by hematite and magnetite, respectively. The data quality is supported by an inverse baked contact test, a B-class reversal test, and the paleomagnetic pole is distinct from any younger poles of the region. Based on the paleomagnetic results, aided by geological evidence, we propose a reconstruction in which the NYB was juxtaposed to southwestern Laurentia in the late Mesoproterozoic and suggest that the late Mesoproterozoic Miaowan-Shimian ophiolite zone in the Yangtze block was likely an extension of the Grenville belt of Laurentia.

Abstract

A M6.8 earthquake struck the High Atlas Mountains in Morocco on 8 September 2023, ending a 63-year seismic silence. We herein attempt to clarify the seismogenic fault and explore the underlying mechanism for this seismic event based on multiple data sets. Utilizing probabilistic Bayesian inversion on interferometric radar data, we determine a seismogenic fault plane centered at a depth of 26 km, striking 251° and dipping 72°, closely aligned with the Tizi n’Test fault system. Given a hypocenter at the Moho depth, the joint inversion of radar and teleseismic data reveals that the rupture concentrates between depths of 12 and 36 km, offsetting the Mohorovičić discontinuity (Moho) at ∼32 km. Considering a strong link between magma activity and failure in lower crust, we propose that the triggering of the earthquake possibly was mantle upwelling that also supports the high topography.

Abstract

The Arabian Sea (AS) hosts the world's thickest and most intense oxygen minimum zone (OMZ), and previous studies have documented a dramatic decline of dissolved oxygen (DO) in the northeastern AS in recent decades. In this study, using the recently released data from Biogeochemical-Argo floats, we found a surprising trend of recovery in deoxygenation within the core region of the OMZ in the AS (ASOMZ) since 2013. The average DO concentration increased by approximately threefold, from ∼0.63 μM in 2013 to ∼1.68 μM in 2022, and the thickness of the ASOMZ decreased by 13%. We find that the weakening of Oman upwelling resulting from the weakening of the summer monsoon is the main driver of oxygenation in the ASOMZ. In addition, the reduction of primary production linked to warming-driven stratification reinforces deoxygenation recovery at depth.

Abstract

Atmospheric rivers (ARs) play a crucial role in the poleward transport of water vapor, and the AR-associated precipitation is a critical component of global water supplies, making it critical that we understand how ARs may change in the future. To approach this issue, integrations of the NASA Goddard Institute for Space Studies global climate model ModelE version 2.1 (GISSE2.1) are employed. Multiple configurations of the model simulating different climates are analyzed: (a) the last-glacial maximum; (b) present day; (c) the end of the 21st century. The thermodynamic and dynamic components of changes to AR frequency are analyzed using a decomposition method. This method utilizes differences in distinct AR seasonal climatology frequencies derived from various vertically integrated water vapor transport (IVT) thresholds to resolve AR frequency into its components. Global mean state changes in poleward AR frequency for different climates are dominated by precipitable water vapor (PWV) changes. A set of idealized cold and warm climates in which present day sea surface temperatures are uniformly changed are considered for a targeted analysis of the south Pacific Ocean basin. For this analysis, frequency and distribution of AR events in the model runs are analyzed by comparing them to changes in the jet stream as well as the Eulerian storm tracks and low-level baroclinicity. Latitudinal shifts in the ARs in the south Pacific Ocean basin using our integrations are not as tightly coupled to these two storm-related climatological metrics in the midlatitudes but fare better on the poleward side of the storm tracks.

Abstract

The detection of preslip, occurring hours to days before a large earthquake, using geodetic measurements has been a major focus in earthquake prediction research. A recent study claims to have detected a preseismic signal interpreted as accelerating slip near the hypocenter of the 2011 great Tohoku-oki earthquake, starting approximately 2 hr before the mainshock. This claim is based on a stacking procedure using GNSS (Global Navigation Satellite System) data. However, a follow-up study demonstrated that the signal disappeared when specific GNSS noise was corrected. Here we utilize tiltmeter records, independent on GNSS, to check whether the claimed preseismic signal is detected using a similar stacking procedure. Our results show no acceleration-like deformation from 2 hr before the mainshock. This indicates that no precursory slip exceeded the noise level of the tilt data, and if any preslip occurred, it was less than 5.0 × 1018 Nm in seismic moment.

Abstract

Marine carbonaceous aerosols, originating from marine and continental sources, are significant global aerosol components. The understanding of marine carbonaceous aerosols is currently limited, especially in the Southern Hemisphere. Furthermore, there is an ongoing debate regarding the contributions of marine fresh and ancient carbon to marine aerosols. To address these gaps, we conducted an extensive investigation utilizing a long-term data set of aerosol samples collected during six Antarctic cruises (28°N–78°S) from 2013 to 2020. Our analysis revealed an average organic carbon (OC) concentration of 1.29 ± 1.15 μg/m3 and an element carbon (EC) concentration of 0.13 ± 0.18 μg/m3 in the samples. These concentrations varied within a range spanning from background marine samples to those impacted by substantial continental transport. Fossil fuel combustion remained the primary source of continental influence in the marine environment, as evidenced by the OC/EC ratio. The δ13CTC value for all samples range from −22.3‰ to −28.4‰, with a mean value of −26.3 ‰. Using a three-endmember isotopic source model, we find that continental carbonaceous aerosols make substantial contributions in the Eastern Indian Ocean (81 ± 4%), while their prevalence is lower in the Southern Ocean (SO) (44 ± 20%). In contrast to mid-latitudes, primary marine aerosol of the SO exhibits a significantly higher contribution from the fresh carbon pool (52 ± 19%). Furthermore, our study suggests that SO sea ice may play a potential role in driving emissions from the fresh carbon pool. These findings contribute to a comprehensive understanding of the effects of carbonaceous aerosols on climate change and the ocean-atmosphere carbon cycle.

Author(s): S. Yu. Gus'kov and G. A. Vergunova

Shock-ignition effect in indirect-drive thermonuclear target is demonstrated on the base of numerical simulations. Thermonuclear gain (in relation to laser pulse energy) of a shock-ignited indirect-drive thermonuclear capsule is obtained, which is 22.5 times higher than that at a traditional spark i…

[Phys. Rev. E 109, 065209] Published Fri Jun 14, 2024

Author(s): Michael L. Nastac, Robert J. Ewart, Wrick Sengupta, Alexander A. Schekochihin, Michael Barnes, and William D. Dorland

This paper investigates, by means of an analytically solvable one-dimensional model, the dissipation in a turbulent, nearly collisionless plasma. When applying a stochastic, external electric field, it is reported that the generalized entropy of the distribution function cascades from large to small scales in position and velocity space, rendering the stochastic heating irreversible.

[Phys. Rev. E 109, 065210] Published Fri Jun 14, 2024

Author(s): Rongzong Huang, Qing Li, and Yu Qiu

In this work, the recent lattice Boltzmann (LB) model with self-tuning equation of state (EOS) [Huang et al., Phys. Rev. E 99, 023303 (2019)] is extended to three dimensions for the simulation of multiphase flows, which is based on the standard three-dimensional 27-velocity lattice and multiple-rel…

[Phys. Rev. E 109, 065306] Published Fri Jun 14, 2024

Abstract

Dimethyl sulfide (DMS) is the largest source of natural sulfur in the atmosphere and undergoes oxidation reactions resulting in gas-to-particle conversion to form sulfate aerosol. Climate models typically use independent chemical schemes to simulate these processes, however, the sensitivity of sulfate aerosol to the schemes used by CMIP6 models has not been evaluated. Current climate models offer oversimplified DMS oxidation pathways, adding to the ambiguity surrounding the global sulfur burden. Here, we implemented seven DMS and sulfate chemistry schemes, six of which are from CMIP6 models, in an atmosphere-only Earth system model. A large spread in aerosol optical depth (AOD) is simulated (0.077), almost twice the magnitude of the pre-industrial to present-day increase in AOD. Differences are largely driven by the inclusion of the nighttime DMS oxidation reaction with NO3, and in the number of aqueous phase sulfate reactions. Our analysis identifies the importance of DMS-sulfate chemistry for simulating aerosols. We suggest that optimizing DMS/sulfur chemistry schemes is crucial for the accurate simulation of sulfate aerosols.

Abstract

In this paper, we examine differences in cloud adjustments (often called rapid adjustments) that occur as a direct result of abruptly increasing the solar constant by 4% or abruptly quadrupling of atmospheric CO2. In doing so, we devise a novel method for calculating the cloud adjustments for the abrupt solar forcing simulations that uses differences between coupled model simulations with abrupt solar and CO2 forcing, in combination with uncoupled, atmosphere-only, abrupt CO2 forced experiments that have prescribed sea-surface temperature. Our main findings are that (a) there are substantial differences in the responses of stratocumulus and cumulus clouds to solar and CO2 forcing, which follow the differences in the direct radiative effect that solar and CO2 forcing have at cloud top, and (b) there are differences in the adjustment of the average optical depth of high clouds to solar and CO2 forcing that we speculate are driven by the differences in the vertical profile of radiative heating and differences in the pattern of sea-surface temperature change (for a fixed global mean temperature). These cloud adjustments contribute significantly to the total net cloud radiative effect, even after 150 years of simulation.

Abstract

The atmospheric large-scale environment determines the occurrence of local extreme precipitation, and it is unclear how climate change affects this relationship. Here we investigate the present-day relationship between large-scale circulation types (CTs) and daily precipitation extremes over Scandinavia and its future change. A 50-member EC-Earth3 large ensemble is used to assess future changes against internal variability. We show that CTs are related to extreme precipitation over the entire domain. The intensity of extreme daily precipitation increases in all seasons in the future climate, generally following the strength of warming in the six different future scenarios considered. However, no significant future change is found in the relationship between extreme precipitation and the CTs in any season or scenario. The results have important implications for applications that rely on the stability of this relationship, such as statistical and event-based dynamical downscaling of future weather and climate predictions and long-term climate projections.

Abstract

We study the statistical features of magnetosphere-ionosphere (M-I) coupling using a two-way M-I model, the GT configuration of the Multiscale Atmosphere Geospace Environment (MAGE) model. The M-I coupling characteristics, such as field-aligned current, polar cap potential, ionospheric Joule heating, and downward Alfvénic Poynting flux, are binned according to the interplanetary magnetic field clock angles over an entire Carrington Rotation event between 20 March and 16 April 2008. The MAGE model simulates similar distributions of field-aligned currents compared to empirical Weimer/AMPS models and Iridium observations and reproduces the Region 0 current system. The simulated convection potential agrees well with the Weimer empirical model and displays consistent two-cell patterns with SuperDARN observations, which benefit from more extensive data sets. The Joule heating structure in MAGE is generally consistent with both empirical Cosgrove and Weimer models. Moreover, our model reproduces Joule heating enhancements in the cusp region, as presented in the Cosgrove model and observations. The distribution of the simulated Alfvénic Poynting flux is consistent with that observed by the FAST satellite in the dispersive Alfvén wave regime. These M-I coupling characteristics are also binned by the Kp indices, indicating that the Kp dependence of these patterns in the M-I model is more effective than the empirical models within the Carrington Rotation. Furthermore, the MAGE simulation exhibits an improved M-I current-voltage relation that closely resembles the Weimer model, suggesting that the updated global model is significantly improved in terms of M-I coupling.

Abstract

Solar wind is an intermediary in energy transfer from the Sun into the Earth's magnetosphere, and is considered as a decisive driver of energetic electron dynamics at the geosynchronous orbit (GEO). Based on machine learning technology, several models driven by solar wind parameters have been established to predict GEO electron fluxes. However, the relative contributions of different solar wind parameters on GEO electron fluxes are still unclear. Recently, a feature attribution method, Deep SHapley Additive exPlanations (Deep SHAP) is proposed to open black boxes of machine learning models. In this study, we use the Deep SHAP method to quantify contributions of different solar wind parameters with an artificial neural network (ANN) model. Backpropagating the prediction results of this ANN model from 2011 to 2020, SHAP values for four solar wind parameters (interplanetary magnetic field (IMF) B Z, solar wind speed, solar wind dynamic pressure, and proton density) are calculated and comprehensively analyzed. The results suggest that solar wind speed with a lag of 1 day is the most important driver. We further investigate relative roles of different parameters in three specific electron fluxes variation events (corresponding to electron fluxes reaching a local maximum, a local minimum, and unchanged, respectively). The results suggest that high solar wind speed and southward IMF B Z (high dynamic pressures) facilitate increases (decreases) of electron fluxes. These findings help reveal the underlying physical mechanisms of GEO electron dynamics and help develop more accurate prediction models for GEO electron fluxes.

Science, Volume 384, Issue 6701, June 2024.

Science, Volume 384, Issue 6701, June 2024.

Science, Volume 384, Issue 6701, June 2024.

Science, Volume 384, Issue 6701, June 2024.

SummaryWe present the first three-dimensional (3-D) upper-mantle conductivity models obtained by an inversion of the satellite-derived tidally-induced magnetic fields (TIMFs). We primarily use the M2 period, but the potential benefit of the O1 period is also inspected. The inverse-problem solution is found using the recently developed frequency-domain, spherical harmonic-finite element method based on the adjoint approach. We tested two different TIMF data sets derived from the satellite measurements of the Swarm mission and two different regularizations; the solution is either required to be sufficiently smooth or reasonably close to the a-priori 3-D conductivity model WINTERC-e Wd-emax. The reconstructed conductivity models are locally compared with the 1-D conductivity profiles from other studies. If we use one of the available TIMF data sets, the smooth reconstructed model gravitates towards Wd-emax and the TIMF-adjusted Wd-emax model is closer to the reference conductivity profiles than the original Wd-emax model. Finally, we use the obtained 3-D conductivity distributions to calculate the corresponding 3-D water distribution in the upper mantle using thermodynamical and compositional models coupled to the electrical-conductivity laboratory measurement of individual mantle constituents.