MAX-DOAS measurements of tropospheric NO2 and HCHO in Munich and the comparison to OMI and TROPOMI satellite observations
Ka Lok Chan, Matthias Wiegner, Carlos Alberti, and Mark Wenig
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2020-35,2020
Preprint under review for AMT (discussion: open, 0 comments)
The manuscript presents 2D MAX-DOAS observations of vertical distribution of aerosol extinction, NO2 and HCHO in Munich. The measured surface aerosol extinction coefficients and NO2 mixing ratios are compared to in-situ monitor data. The NO2 and HCHO data are subsequently used to validate satellite measurements. The MAX-DOAS measurements are also used to investigate the spatio-temporal characteristic of NO2 and HCHO in Munich.
Validation of tropospheric NO2 column measurements of GOME-2A and OMI using MAX-DOAS and direct sun network observations
Gaia Pinardi, Michel Van Roozendael, François Hendrick, Nicolas Theys, Nader Abuhassan, Alkiviadis Bais, Folkert Boersma, Alexander Cede, Jihyo Chong, Sebastian Donner, Theano Drosoglou, Udo Frieß, José Granville, Jay R. Herman, Henk Eskes, Robert Holla, Jari Hovila, Hitoshi Irie, Yugo Kanaya, Dimitris Karagkiozidis, Natalia Kouremeti, Jean-Christopher Lambert, Jianzhong Ma, Enno Peters, Ankie Piters, Oleg Postylyakov, Andreas Richter, Julia Remmers, Hisahiro Takashima, Martin Tiefengraber, Pieter Valks, Tim Vlemmix, Thomas Wagner, and Folkard Wittrock
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2020-76,2020
Preprint under review for AMT (discussion: open, 0 comments)
We validate several GOME-2 and OMI tropospheric NO2 products with 23 MAX-DOAS and 16 direct sun instruments distributed worldwide. We highlight large horizontal inhomogeneities at several sites affecting the validation results and we propose a method to quantify and correct for it. We show that the application of such correction reduces the satellite underestimation in almost all heterogeneous cases, but a negative bias remains over the MAX-DOAS + direct sun network ensemble for both satellites.
Testing the near-field Gaussian plume inversion flux quantification technique using unmanned aerial vehicle sampling
Adil Shah, Joseph R. Pitt, Hugo Ricketts, J. Brian Leen, Paul I. Williams, Khristopher Kabbabe, Martin W. Gallagher, and Grant Allen
Atmos. Meas. Tech., 13, 1467–1484, https://doi.org/10.5194/amt-13-1467-2020, 2020
Methane is a potent greenhouse gas, with large flux uncertainties from facility-scale sources, such as natural gas extraction infrastructure. A recently developed flux quantification method was successfully tested by flying an unmanned aerial vehicle (UAV) downwind of 22 controlled atmospheric methane releases. The UAVs were used to derive high-precision atmospheric methane measurements. The UAV methodology was successful in both detecting the release and providing a rough flux estimate.
InnFLUX – an open-source code for conventional and disjunct eddy covariance analysis of trace gas measurements: an urban test case
Marcus Striednig, Martin Graus, Tilmann D. Märk, and Thomas G. Karl
Atmos. Meas. Tech., 13, 1447–1465, https://doi.org/10.5194/amt-13-1447-2020, 2020
The current work summarizes a long-term effort to provide an open-source code for the analysis of turbulent fluctuations of trace gases in the atmosphere by eddy covariance and disjunct eddy covariance, with a special focus on reactive gases that participate in atmospheric chemistry. The performance of the code is successfully evaluated based on measurements of minute fluxes of non-methane volatile organic compounds into the urban atmosphere.
The 2018 fire season in North America as seen by TROPOMI: aerosol layer height intercomparisons and evaluation of model-derived plume heights
Debora Griffin, Christopher Sioris, Jack Chen, Nolan Dickson, Andrew Kovachik, Martin de Graaf, Swadhin Nanda, Pepijn Veefkind, Enrico Dammers, Chris A. McLinden, Paul Makar, and Ayodeji Akingunola
Atmos. Meas. Tech., 13, 1427–1445, https://doi.org/10.5194/amt-13-1427-2020, 2020
This study looks into validating the aerosol layer height product from the recently launched TROPOspheric Monitoring Instrument (TROPOMI) for forest fire plume through comparisons with two other satellite products, and interpreting differences due to the individual measurement techniques. These satellite observations are compared to predicted plume heights from Environment and Climate Change's air quality forecast model.
Shipborne MAX-DOAS measurements for validation of TROPOMI NO2 products
Ping Wang, Ankie Piters, Jos van Geffen, Olaf Tuinder, Piet Stammes, and Stefan Kinne
Atmos. Meas. Tech., 13, 1413–1426, https://doi.org/10.5194/amt-13-1413-2020, 2020
The comparison of shipborne MAX-DOAS and TROPOMI NO2 products is important for the evaluation of the TROPOMI products. The ship cruises were mainly over remote oceans, thus we only measured background tropospheric NO2. Stratospheric NO2 was measured more accurately because there was almost no contamination from tropospheric NO2. We found that the TROPOMI stratospheric NO2 vertical column densities were slightly higher than the MAX-DOAS measurements.
Quality controls, bias, and seasonality of CO2 columns in the Boreal Forest with OCO-2, TCCON, and EM27/SUN measurements
Nicole Jacobs, William R. Simpson, Debra Wunch, Christopher W. O'Dell, Gregory B. Osterman, Frank Hase, Thomas Blumenstock, Qiansi Tu, Matthias Frey, Manvendra K. Dubey, Harrison A. Parker, Rigel Kivi, and Pauli Heikkinen
Atmos. Meas. Tech. Discuss., https//doi.org/10.5194/amt-2019-505,2020
Preprint under review for AMT (discussion: open, 0 comments)
The Boreal forest is the largest seasonally-varying biospheric carbon dioxide exchange region on Earth. This region is also undergoing amplified climate warming leading to concerns about the potential for altered regional carbon exchange. Satellite missions such as the orbiting carbon observer-2 (OCO-2) project can measure CO2 abundance over the Boreal forest, but need validation for assurance of accuracy. Therefore, we carried out ground-based validation of OCO-2 CO2 data at three locations.
Validation of tropospheric NO2 column measurements of GOME-2A and OMI using MAX-DOAS and direct sun network observations
Gaia Pinardi, Michel Van Roozendael, François Hendrick, Nicolas Theys, Nader Abuhassan, Alkiviadis Bais, Folkert Boersma, Alexander Cede, Jihyo Chong, Sebastian Donner, Theano Drosoglou, Udo Frieß, José Granville, Jay R. Herman, Henk Eskes, Robert Holla, Jari Hovila, Hitoshi Irie, Yugo Kanaya, Dimitris Karagkiozidis, Natalia Kouremeti, Jean-Christopher Lambert, Jianzhong Ma, Enno Peters, Ankie Piters, Oleg Postylyakov, Andreas Richter, Julia Remmers, Hisahiro Takashima, Martin Tiefengraber, Pieter Valks, Tim Vlemmix, Thomas Wagner, and Folkard Wittrock
Atmos. Meas. Tech. Discuss., https//doi.org/10.5194/amt-2020-76,2020
Preprint under review for AMT (discussion: open, 0 comments)
We validate several GOME-2 and OMI tropospheric NO2 products with 23 MAX-DOAS and 16 direct sun instruments distributed worldwide. We highlight large horizontal inhomogeneities at several sites affecting the validation results and we propose a method to quantify and correct for it. We show that the application of such correction reduces the satellite underestimation in almost all heterogeneous cases, but a negative bias remains over the MAX-DOAS + direct sun network ensemble for both satellites.
Testing the near-field Gaussian plume inversion flux quantification technique using unmanned aerial vehicle sampling
Adil Shah, Joseph R. Pitt, Hugo Ricketts, J. Brian Leen, Paul I. Williams, Khristopher Kabbabe, Martin W. Gallagher, and Grant Allen
Atmos. Meas. Tech., 13, 1467–1484, https://doi.org/10.5194/amt-13-1467-2020, 2020
Methane is a potent greenhouse gas, with large flux uncertainties from facility-scale sources, such as natural gas extraction infrastructure. A recently developed flux quantification method was successfully tested by flying an unmanned aerial vehicle (UAV) downwind of 22 controlled atmospheric methane releases. The UAVs were used to derive high-precision atmospheric methane measurements. The UAV methodology was successful in both detecting the release and providing a rough flux estimate.
InnFLUX – an open-source code for conventional and disjunct eddy covariance analysis of trace gas measurements: an urban test case
Marcus Striednig, Martin Graus, Tilmann D. Märk, and Thomas G. Karl
Atmos. Meas. Tech., 13, 1447–1465, https://doi.org/10.5194/amt-13-1447-2020, 2020
The current work summarizes a long-term effort to provide an open-source code for the analysis of turbulent fluctuations of trace gases in the atmosphere by eddy covariance and disjunct eddy covariance, with a special focus on reactive gases that participate in atmospheric chemistry. The performance of the code is successfully evaluated based on measurements of minute fluxes of non-methane volatile organic compounds into the urban atmosphere.
The 2018 fire season in North America as seen by TROPOMI: aerosol layer height intercomparisons and evaluation of model-derived plume heights
Debora Griffin, Christopher Sioris, Jack Chen, Nolan Dickson, Andrew Kovachik, Martin de Graaf, Swadhin Nanda, Pepijn Veefkind, Enrico Dammers, Chris A. McLinden, Paul Makar, and Ayodeji Akingunola
Atmos. Meas. Tech., 13, 1427–1445, https://doi.org/10.5194/amt-13-1427-2020, 2020
This study looks into validating the aerosol layer height product from the recently launched TROPOspheric Monitoring Instrument (TROPOMI) for forest fire plume through comparisons with two other satellite products, and interpreting differences due to the individual measurement techniques. These satellite observations are compared to predicted plume heights from Environment and Climate Change's air quality forecast model.
Shipborne MAX-DOAS measurements for validation of TROPOMI NO2 products
Ping Wang, Ankie Piters, Jos van Geffen, Olaf Tuinder, Piet Stammes, and Stefan Kinne
Atmos. Meas. Tech., 13, 1413–1426, https://doi.org/10.5194/amt-13-1413-2020, 2020
The comparison of shipborne MAX-DOAS and TROPOMI NO2 products is important for the evaluation of the TROPOMI products. The ship cruises were mainly over remote oceans, thus we only measured background tropospheric NO2. Stratospheric NO2 was measured more accurately because there was almost no contamination from tropospheric NO2. We found that the TROPOMI stratospheric NO2 vertical column densities were slightly higher than the MAX-DOAS measurements.
Quality controls, bias, and seasonality of CO2 columns in the Boreal Forest with OCO-2, TCCON, and EM27/SUN measurements
Nicole Jacobs, William R. Simpson, Debra Wunch, Christopher W. O'Dell, Gregory B. Osterman, Frank Hase, Thomas Blumenstock, Qiansi Tu, Matthias Frey, Manvendra K. Dubey, Harrison A. Parker, Rigel Kivi, and Pauli Heikkinen
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2019-505,2020
Preprint under review for AMT (discussion: open, 0 comments)
The Boreal forest is the largest seasonally-varying biospheric carbon dioxide exchange region on Earth. This region is also undergoing amplified climate warming leading to concerns about the potential for altered regional carbon exchange. Satellite missions such as the orbiting carbon observer-2 (OCO-2) project can measure CO2 abundance over the Boreal forest, but need validation for assurance of accuracy. Therefore, we carried out ground-based validation of OCO-2 CO2 data at three locations.
Evaluation of satellite-based aerosol datasets and the CAMS reanalysis over the ocean utilizing shipborne reference observations
Jonas Witthuhn, Anja Hünerbein, and Hartwig Deneke
Atmos. Meas. Tech., 13, 1387–1412, https://doi.org/10.5194/amt-13-1387-2020, 2020
Reliable reference measurements over ocean are essential for the evaluation and improvement of satellite- and model-based aerosol datasets. Here, a uniqe set of shipborne reference aerosol products obtained from Microtops sunphotometer and GUVis-3511 shadowband radiometer observations are compared to aerosol products from the MODIS and SEVIRI satellite sensors, and the CAMS reanalysis over the Atlantic Ocean. The present evaluation highlights the importance of an aerosol-type based analysis.
A Phase Separation Inlet for Droplets, Ice Residuals, and Interstitial Aerosols
Libby Koolik, Michael Roesch, Lesly J. Franco Deloya, Chuanyang Shen, A. Gannet Hallar, Ian B. McCubbin, and Daniel J. Cziczo
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2020-42,2020
Preprint under review for AMT (discussion: open, 0 comments)
The phaSe seParation Inlet for Droplets icE residuals and inteRstitial aerosols (SPIDER) combines an omni-directional inlet, a Large-Pumped Counterflow Virtual Impactor, a flow tube evaporation chamber, and a Pumped Counterflow Virtual Impactor to separate droplets, ice crystals, and interstitial aerosols for simultaneous sampling. This new inlet for studying mixed-phase clouds is described here, with laboratory verification tests and a deployment at a mountain-top research facility.
Evaluation of satellite-based aerosol datasets and the CAMS reanalysis over the ocean utilizing shipborne reference observations
Jonas Witthuhn, Anja Hünerbein, and Hartwig Deneke
Atmos. Meas. Tech., 13, 1387–1412, https://doi.org/10.5194/amt-13-1387-2020, 2020
Reliable reference measurements over ocean are essential for the evaluation and improvement of satellite- and model-based aerosol datasets. Here, a uniqe set of shipborne reference aerosol products obtained from Microtops sunphotometer and GUVis-3511 shadowband radiometer observations are compared to aerosol products from the MODIS and SEVIRI satellite sensors, and the CAMS reanalysis over the Atlantic Ocean. The present evaluation highlights the importance of an aerosol-type based analysis.
A Phase Separation Inlet for Droplets, Ice Residuals, and Interstitial Aerosols
Libby Koolik, Michael Roesch, Lesly J. Franco Deloya, Chuanyang Shen, A. Gannet Hallar, Ian B. McCubbin, and Daniel J. Cziczo
Atmos. Meas. Tech. Discuss., https//doi.org/10.5194/amt-2020-42,2020
Preprint under review for AMT (discussion: open, 0 comments)
The phaSe seParation Inlet for Droplets icE residuals and inteRstitial aerosols (SPIDER) combines an omni-directional inlet, a Large-Pumped Counterflow Virtual Impactor, a flow tube evaporation chamber, and a Pumped Counterflow Virtual Impactor to separate droplets, ice crystals, and interstitial aerosols for simultaneous sampling. This new inlet for studying mixed-phase clouds is described here, with laboratory verification tests and a deployment at a mountain-top research facility.
Retrieval of eddy dissipation rate from derived equivalent vertical gust included in Aircraft Meteorological Data Relay (AMDAR)
Soo-Hyun Kim, Hye-Yeong Chun, Jung-Hoon Kim, Robert D. Sharman, and Matt Strahan
Atmos. Meas. Tech., 13, 1373–1385, https://doi.org/10.5194/amt-13-1373-2020, 2020
We retrieve the eddy dissipation rate (EDR) from the derived equivalent vertical gust included in the Aircraft Meteorological Data Relay data for more reliable and consistent observations of aviation turbulence globally with the single preferred EDR metric. We convert the DEVG to the EDR using two methods (lognormal mapping scheme and best-fit curve between EDR and DEVG), and the DEVG-derived EDRs are evaluated against in situ EDR data reported by US-operated carriers.
Evaluation of UV Aerosol Retrievals from an Ozone Lidar
Shi Kuang, Bo Wang, Michael J. Newchurch, Paula Tucker, Edwin W. Eloranta, Joseph P. Garcia, Ilya Razenkov, John T. Sullivan, Timothy A. Berkoff, Guillaume Gronoff, Liqiao Lei, Christoph J. Senff, Andrew O. Langford, Thierry Leblanc, and Vijay Natraj
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2020-40,2020
Preprint under review for AMT (discussion: open, 0 comments)
Ozone lidar is a state-of-art remote sensing instrument to measure atmospheric ozone concentration with high spatio-temporal resolution. In this study, we show that an ozone lidar can also provide reliably aerosol measurements with high resolution by using the collocated data taken by the ozone lidar and an aerosol lidar. This means that ozone lidars are capable of providing simultaneous ozone and aerosol measurements.
Retrieval of eddy dissipation rate from derived equivalent vertical gust included in Aircraft Meteorological Data Relay (AMDAR)
Soo-Hyun Kim, Hye-Yeong Chun, Jung-Hoon Kim, Robert D. Sharman, and Matt Strahan
Atmos. Meas. Tech., 13, 1373–1385, https://doi.org/10.5194/amt-13-1373-2020, 2020
We retrieve the eddy dissipation rate (EDR) from the derived equivalent vertical gust included in the Aircraft Meteorological Data Relay data for more reliable and consistent observations of aviation turbulence globally with the single preferred EDR metric. We convert the DEVG to the EDR using two methods (lognormal mapping scheme and best-fit curve between EDR and DEVG), and the DEVG-derived EDRs are evaluated against in situ EDR data reported by US-operated carriers.
